My guess would be limitations of the spectral purity of the local oscillator. (I haven't seen the hardware design.)
The two ranges suggest that it works similarly to the NanoVNA: a signal source is being used to generate frequencies up to 320 MHz, and the third harmonic of that source is used for the higher frequency range. Enabling an even higher range to 1.5 GHz would require using the fifth harmonic of the LO or switching to a different LO design.
As those of you have used the original NanoVNA (probably just about everybody here) know, the dynamic range is severely limited on the highest range, the one that extends coverage to 1.5 GHz. That's because you're going way beyond what the Si5351A is intended to do. It is still useful for many applications of a VNA, but a dynamic range of 40dB is too low for most of the things you use a spectrum analyzer for. It's not enough, for example, to use it to detect non-compliance with FCC spectral purity requirements for transmitters. TinySA will not be a lab grade instrument and as such is probably not adequate for full compliance testing; you'll still need verification by a better equipped lab for that. But it can serve as a way of finding non-compliant designs.